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Completed TRL 3 (started at 2, targeting 3)
The proposed work is to develop a novel solid electrolyte (NSE) by harnessing superior self-assembly ability of a multi-segmented polymer and conformal polymer electrografting with desired molecules/functional groups of promoting fast ionic transport and/or formation of stabilized solid electrolyte interphase, to address the low ionic conductivity and mitigate the interfacial issues. This NSE along with the new fabrication process enables high ionic conductivity, minimizes/mitigates the interfacial impedances between NSE/Li metal anode and NSE/high capacity cathode, and enables Li metal safely cycling. In addition, this polymer has offered a reversible thermodynamic transition with no volume change, which can potentially be used as internal self-thermal management
Introducing the Novel Solid Electrolyte and the accompanying internal thermal management leads to a new generation of battery designs, no longer requiring external safety and thermal management accessories, and provides simplified system designs with significantly increased energy density.
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